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Quantum-Enhanced Nonlinear Spectroscopy
Frank Schlawin
出版
Springer
, 2016-09-10
主題
Science / Physics / Quantum Theory
Science / Physics / Optics & Light
Science / Chemistry / Physical & Theoretical
Science / Spectroscopy & Spectrum Analysis
Science / Chaotic Behavior in Systems
Science / Physics / General
Science / Chemistry / Analytic
ISBN
3319443976
9783319443973
URL
http://books.google.com.hk/books?id=930EDQAAQBAJ&hl=&source=gbs_api
EBook
SAMPLE
註釋
This thesis focuses on nonlinear spectroscopy from a quantum optics perspective. First, it provides a detailed introduction to nonlinear optical signals; starting from Glauber’s photon counting formalism, it establishes the diagrammatic formulation, which forms the backbone of nonlinear molecular spectroscopy. The main body of the thesis investigates the impact of quantum correlations in entangled photon states on two-photon transitions, with a particular focus on the time-energy uncertainty, which restricts the possible simultaneous time and frequency resolution in measurements. It found that this can be violated with entangled light for individual transitions. The thesis then presents simulations of possible experimental setups that could exploit this quantum advantage. The final chapter is devoted to an application of the rapidly growing field of multidimensional spectroscopy to trapped ion chains, where it is employed to investigate nonequilibrium properties in quantum simulations.