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Gaseous Vanadium, Vanadium Oxide and Hydroxide Clusters
Sandra Feyel
其他書名
From Clusters to Model Catalysts
出版Logos Verlag Berlin GmbH, 2008
主題Science / Chemistry / General
ISBN38325205119783832520519
URLhttp://books.google.com.hk/books?id=9zvPQAexCsUC&hl=&source=gbs_api
EBookSAMPLE
註釋The present work explores the reactivities of gaseous vanadium, vanadium-oxide, and oxovanadium-hydroxide clusters toward methanol and small hydrocarbons. Various means of mass-spectrometric techniques, isotopic labeling studies, infrared photodissociation spectroscopy, and complementary DFT-calculations are employed for this purpose. Additionally, the hydrogen-atom abstraction process from methane by polynuclear metal oxides is discussed. This work contributes to a better understanding of the metal-oxide cluster's catalytic activity on a molecular scale.